Thermodynamic Optimization of TmCl3-ACl （A = Na, K, Rb, Cs）Phase Diagrams
摘要
From the measured phase equilibria data and experimental thermochemical properties, the TmCl3-ACl (A=Na, K, Rb, Cs) phase diagrams were optimized and calculated using the CALPHAD technique. For describing the Gibbs energies of the liquid phase in these systems, the new modified quasichemical model in the pair-approximation for short-range ordering was used. A set of thermodynamic functions was optimized and gotten based on an interactive computer-assisted analysis. The calculated phase diagrams and thermodynamic data are self-consistent.
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叶信宇, Jing Zhang, 孙益民, 等. Thermodynamic Optimization of TmCl3-ACl （A = Na, K, Rb, Cs）Phase Diagrams[J]. Acta Scientiarum Naturalium Universitatis Sunyatseni, 2005.
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